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🔋 Microenvironment‐Regulated Interfacial Reconstruction Enables High‐Performance Direct Regeneration of Spent LiFePO 4 Cathodes

📝 این مقاله با تنظیم ریزمحیط و بازسازی بین‌سطحی، بازتولید مستقیم کارآمد کاتدهای LiFePO4 مستعمل را با پایداری چرخه‌ای عالی ارائه می‌دهد.

📚 Journal: Advanced Functional Materials #AdvancedFunctionalMaterials
📅 Date: 2026-10-06
🔬 Research Article

💡 Novelty & Significance:
This work introduces a microenvironment regulation strategy using dicyandiamide and lithium orotate to synergistically remove surface impurities and reconstruct interfaces during direct regeneration of spent LiFePO₄. It enables efficient relithiation with in situ nitrogen-doped carbon layers, achieving 90.9% capacity retention after 1000 cycles at 5 C, offering a techno-economically viable route for closed-loop battery recycling.

🔗 10.1002/adfm.78704

🏷 LiFePO4 cathode · direct regeneration · spent batteries · interfacial reconstruction · nitrogen doping
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